Brooklyn Industries, though I actually prefer their hoodie/jacket selection, for originality and quality.

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honestly Das Monk - www.dasmonk.com has by far the best printed tees going around. The fits are amazing too. I have a heap of them.

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Go to Rumplo.com
They feature shirts from ALL OVER and they link over to the so you can buy them.

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I knew that I wouldn't be the first to recommend Threadless for this question. Try them out, though. Artists from all over submit designs, so there is an enormous selection of t-shirts that you'll never find in a store. threadless.com

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www.bloodisthenewblack.com has some pretty cool independent artist t's

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Might be a long shot, but Turntable Lab has a ton of cool shirts...

Turntable Lab

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Lots of good suggestions.
Some really nice tees at Ugmonk as well.

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